“Psycho Soldier” by Akira Yamaoka, from the No More Heroes 2: Desperate Struggle soundtrack. I’m digging this song a lot, but it has the unfortunate side effect of reminding me of the song from SNK’s game Psycho Soldier, which you’re going to have to listen to now, in both English:

and Japanese:

We all have to listen to them now! It’s out of my hands!

Buy: No More Heroes 2: Desperate Struggle ($46.99)

See also: “Twilight” by Akira Yamaoka, “The Year Of The Travis 2010”, Unlockable Bizarre Jelly 5 anime intro